SB 191 L41 m^T* >^^->^. :^> ^i.■ #■. -^.^ ^^>^ 1 1 f\ ALBERT R. MANN LIBRARY New York State Colleges OF Agriculture and Home Economics AT Cornell University Cornell University Library The original of tiiis book is in tine Cornell University Library. There are no known copyright restrictions in the United States on the use of the text. http://www.archive.org/details/cu31924003370586 ON SOME POINTS IN THE COMPOSITION OF WHEA.T-GMIN, ITS PEODUCTS IN THE MILL, AND EEEAD. BT J. B. LAWES, F.K.S., F.C.S, jlnd J. H. GILBERT, Ph. D., F.C.S. LONDON: I'RINTEI) BT HAEEISOK AND SONS, ST, MARTIN'S LANE, W.C. 185!;, ON SOME POINTS IN THE COMPOSITION OF WHEAT-GRAIN, ITS PEO- DUCTS IN THE MILL AND BEEAD, By J. B. LAWES, P.E.S., F.C.S., and J. H. GILBERT, Ph. D., F.C.S. The composition of the grain yielding the most important article of human food in temperate climates^ its yield of valuable products, and the varying composition either of the grain itself, or of these products, according to the conditions of growth, or the circum- stances of after preparation, are subjects worthy the attention equally of states and of men of science. Accordingly we find, that a chemical examination of wheat-grain and its products, has from time to time been undertaken by chemists of repute ; sometimes as a matter of private investigation, and at others of public inquiry .; and almost as numerous as the names of the experimenters, are the special lines of research which they have selected. We are indebted to Beccaria for the first notice, more than a century ago, of the gluten in wheat. Among the earlier investi- gators of the subsequent period, are, Proust, Vauquelin, De Saussure and Vogel, who have examined the proximate principles, and some of the changes to which they are subject, in various descriptions of wheat, of flour, or of bread. M. Bous- singault has somewhat elaborately studied various branches of the subject more recently; and we are indebted to Dumas, B 2 LAWES AND GILBERT Payen, Jolinston, and Dr. R. D. Thomson for original, as well as a considerable amount of collected information. The most recent; on some points the most detailed, and from advance m methods, perhaps on some also the most rehable, are the results ofM. Peligot in 1S49, on the proximate constitution of various kinds of wheat, and of M. Mi lion in 1849 and 1854, on some- what similar points. Lastly, in 1853 M. Poggiale, and in 1855 Dr. Maclagan, have given the results of their investigations on the characters and composition of bread. Besides these more general investigations, we have had in recent times many special inquiries connected with our subject. Thus, M. Boussingault has given us analyses of the ashes of wheat ; and many other such analyses have been made in Ger- many, and elsewhere, since the first appearance, in 1840, of Baron Liebig's work on "Chemistry in its Applications to Agriculture and Physiology." In this country, Mr. Way has given us the most extensive series of wheat-grain-ash analyses, his list including those of 26 specimens or descriptions. The plan of our own investigation, which unfortunately has been much less perfectly filled up than we at first intended, was entered upon more than a dozen years ago, and was devised with reference to the following points : — 1st. The influence of varying characters of season, and of vari- ous manuring, upon the organic and mineral composition of wheat grain. 2ndly. The characters of varieties, especially in relation to their adaptation, and the qualities they then develop, under the influence of broader distinctions as to locality, altitude, latitude, and vary- ing climatic circumstances generally. It is in the second branch of the inquiry that we have fallen the furthest short of our intentions. With a view to its prosecution, a journey through the chief corn growing districts of Europe, com- mencing at the northernmost point at which wheat is grown suc- cessfully, was about to be undertaken in 1848; but the social dis- turbances on the continent at that period, necessarily prevented it. The plan proposed was — to collect information, as to the geological and meteorological characters of the various localities, as to the mode of culture, and as to the general acreage yield, both in straw and grain ; and lastly, to procure characteristic specimens for chemical examination at home. Failing entirely in the execution of this design, the Exhibition of 1851 was looked forward to as an oppor- ON THE COMPOSITION OF WHEAT-GRAIN, &0. 3 tunity for procTiring spepimens not only of wheat, but of other vegetable products, and perhaps also important particulars of their growth, from various countries and climates. Such, however, was the division of authority, and such the alleged preference given to public institutions in such matters, that, whether the latter bene- fited or not, the collection which we, as private individuals, were enabled to make, was entirely inadequate to our object. From these difficulties it is, that our second main object of inquiry was necessarily to a great extent abandoned ; and chiefly for this rea- son, but partly owing to the pressure of other subjects ; the first or more limited or local branch of the investigation has in recent years been but imperfectly followed up. And, as it is probable that it must for some time remain so, it has been thought desirable thus to put on record the results already obtained ; hoping that they may serve the double purpose, of confirming or adding to previously existing knowledge, and of indicating to others ■ the points most requiring further study. The following is a brief outline of the plan of investigation which has yielded the results which we have now to lay before the Society. From the season 1843-4, up to the present time, wheat has been growing in the same field continuously, both without manure, by ordinary, and by various chemical manures. As a general rule, the same description of manure has succeeded year after year on the same plot of land. The amount of produce, corn, straw, and chaff, and its characters as to weight per bushel, &c., have in every case, been carefully ascertained and recorded. Samples from each plot — ;both grain and straw^— have also been collected every year. Of each of these samples two weighed por- tions are coarsely ground ; the dry matter determined at a tempera- ture of 213° ; and the ash by burning on sheets of platinum, in cast iron muffles arranged for that purpose.* Other weighed por- tions of grain and straw are partially dried, so as to prevent their decomposition ; and in this state they are preserved for any exami- nation of their organic constituents. By this course of procedure, ,a vast mass of results has been obtained, illustrating the influence of season and manuring, upon the percentage of dry substance, and of mineral constituents, in the produce. In selected cases, the nitrogen in the grain, and in the straw, has been determined. * The dry matter and ash, were not determined In such complete series in the earlier years, as, ia the later. b2 4 LAWES AXD GILBERT A summary table of these dry matter, ash, and nitrogen results, will be given below. In from twenty to thirty cases complete analyses of the grain-ashes have been made, and the results of these will be given in full. Besides the experiments above described, in selected cases, chiefly from the produce of the earlier years of the field experi- ments, it was sought to ascertain the comparative yield of flour, and also the characters of the flour, of grain grown by different manures in the same season, or by the produce of different sea- sons. The colonist's steel handmill was first had recourse to for this purpose. But it was soon found, that it was extremely diflS- cult so to regulate the machine, as to secure uniform action upon the difl^erent grains ; and it was further found, that the grain, and especially the bran, was cut up rather than crushed, so as to leave too much of fiour in the portion separated as bran, and too much of . bran in that separated as flour ; and hence the results were not sufficiently comparable with those of the ordinary mill, Arrange- iQcnts were therefore made for prosecuting the inquiry at a flour mill in the neighbourhood, worked by water power. Weighed quantities of the selected samples (from 125 to 250 lbs. each), were passed through the stones, and the " meal" thus obtained, through the dressing machine, under our own personal superintendence ; great care being taken to clear from the diff'erent parts of the apparatus the whole of one lot, before another was commenced upon. The yield in the dressing machine of each of the diflferent products was ascertained, and its percentage in relation to the total grain or its " meal," has been calculated. Portions of each of these products have had their drj^ matter (at 212°), and their mineral matter (by burning on platinum), determined. The per- centage of nitrogen in a few selected series — from the flnest flour down to the coarsest bran — has also been estimated ; and in the same cases, the amounts of one or two of the more important constituents of the ash have also been determined. The results of these dry matter, ash, >> ''"^"-gen, and constituent of ash deter- minations, in the series of diflerent products obtained in the mill, will be given in tables further on. The original design, was to complete the examination of the mill products, by determining in several series cf them, the per- centage of each of their proximate organic principles ; and also the amount and composition of mineral matters, associated with ox THE COMPOSITION OF WHEAT-GEAINj &C. 5 them respectively. It was hoped, by this latter inquiry, to; obtain, important collateral information, bearing upon the influence of various constituents upon the healthy and special development of the plant. Although, however, specimens of the flour are pre- served for this purpose, as well as the ashes of each crude pro- duct, it is feared that this subject cannot be proceeded with, at least for a considerable time to come. Portions of the different products of the dressing machine (including more or less of the finest flour, of the more granular, or of the more branny particles respectively), from grains of somewhat various history of growth, have been experimented upon to ascertain their comparative bread-making qualities ; and these results, together with a few examinations of baker's bread, and a discussion of the results of other experimenters, as to the yield of bread from a given amount of flour, and the percentage of water and of nitrogen in the former, will be given below. With this short outline of the plan of investigation which has been pursued, we proceed now to a discussion of the results which have been obtained. In Table I. are given, in the first four columns, certain pro- minent characters of the produce of each of ten years of the suc- cessive growth of wheat as above described. The items are : — The total produce per acre (corn and straw), in lbs. ; The per cent, of corn in the total produce ; The per cent, of dressed corn in the total corn ; and, The weight per bushel of dressed corn in lbs. The figure given for each year, generally represents the average of about 40 cases; and the characters enumerated are the best which can be given in a summary and numerical form, to indicate the more or less favourable condition of the respec- tive seasons for the healthy development of the crop, and the perfect maturation of the grain. In the second set of three columns are given, side by side with the general characters just described, the percentages in the grain of each year — Of dry substance ; Of ash in dry substance ; and. Of nitrogen in dry substance ; the two former items being in most cases the average of 30 to 40 cases in each year; but the per cent, of nitrogen, is in each instance, the mean of a few selected cases only. LAWES AND GILBEET In the third set of three columns, are given similar particu- lars relating to the composition of the straw. The percentages of dry substance and of ash in the straw, are however not the averages of so many cases in each year, as are those for the corn ; and the determinations of nitrogen in the straw, have also been made in fewer cases than in the grain. It will thus be seen, that the table affords a summary view of a really enormous amount of experimental result, and we ought to be able by its means to discover, at least the broad and characteristic effects of varying seasons, upon the compo- sition of the crop.* This indeed is all we could hope to attain, in such a mere outline and general treatment of the subject as is appropriate to our present purpose. TABLE I. General Summary. Particulars of the Frodace. Composition of Gaain. Composition of Straw. Total Per cent. Weight corn and Per cent. dressed per bushel of dressed Per cent. Per cent Per cent. Per cent. Percent. Percent. Harvests straw per acre corn in total com m total dry aeh in nitrogen dry ash in nitrogen in lbs. produce. com. corn in lbs. (212°) dry. in dry. (212°.) dry. in dry. 1845 5645 33-1 90-1 S6-7 80-8 1-91 2-25 7-06 0-92 1846 4114 43-1 93-2 63-1 84-3 1-96 2-15 ,i 602 0-67 1847 .5221 36-4 93-6 62-0 2-30 .. 6-56 0-73 1848 4517 36-7 89-0 68-5 80-3 202 2-39 .. 7-24 0-78 1849 5321 40-9 96-5 63-5 83-1 1-84 1-94 82-6 6-17 0-82 1860 5496 33-6 94-3 60-9 84-4 1-99 2-15 84-4 5-88 0-87 1851 5279 38-2 92-1 62-6 84-2 1-89 1-98 84-7 6-88 0-78 1852 4299 31'6 92-1 56-7 83-2 2-00 2-38 82-6 6-53 0-79 1853 3932 25-1 85-9 50'2 80-8 2-24 2-35 81-0 6-27 1-20 1854 6803 35-8 95-6 61-4 84-9 1-93 2-14 83-7 5-08 0-69 Means 5053 • 36-4 92-1 59-6 82-9 1-98 2-20 83-2 6-17 0-82 Leaving then out of view all minor points, and confining our- selves to our already defined object — namely, that of ascertaining the general direction of the influence of variation of season upon the composition of the wheat crop — we cannot fail to see, that wherever the three items indicating the quality of the produce * It should be stated, that up to 1848 inclusive, the description of wheat was the Old Bed Lammas ; from 1849 to 1852 inclusire, it was the Bed Cluster, and since that time the Eostook. The variations, according to season, both in the characters and composition of the pToducei, arc, however, very marked *ithin the period of growth of each separate description. ON THE COMPOSITION OF WHEATtGKAIN, &0. 7 markedly distinguish the crop as favourably developed, we have a general tendency to a high percentage of dry substance, and to a low percentage both of mineral matter, and of nitrogen, in that dry substance. This generalization is more especially applicable to the grain > but with some exceptions, mostly explicable on a detailed consideration of the circumstances and degree of its deve- lopment^ it applies to a great extent to the straw also. Let us take in illustration the extreme cases in the table. The seasons of ,1846> 1849, and 1851, with in the cases of the two latter large produce .also, give us the best proportion of corn in total produce, more than the average proportion of dressed corn in total com, and the highest weight per bushel — a very significant character. With this cumulative evidence as to the relatively favourable development and maturation of these crops, we find the grain in two of the cases, to be among the highest in percentage of dry matter ; and in the third (1849), though not so high as we should have expected, it is still above the average. The per- centages of mineral matter and of nitrogen in the dry substance of the grain, are at the same time, in these three cases, the lowest in the series. The seasons of 1850 and 1854 again, with large amounts of produce, yielded also very fairly developed grain ; and coincidently they afford a high percentage of dry substance, and lower percentages both of mineral matter, and of nitrogen, in that dry substance, than the cases of obviously inferior maturation. With some exceptions, it wiU be seen, that the straws also of these 5 betier years, give a tendency to low percentages both of mineral matter and of nitrogen in their dry substance- Turning now to the converse aspect, the season of 1853, shows itself in the general characters of the produce, to have been in every respect the least favourable to the crop ; and it ishould be added that in this instance (as well as in 1845 to which we shall next refer), the seed was not sown until the spring. In 1853 the produce of grain was small as well as very bad in quality ; and with these characters, we have in thd grain nearly the lowest per- centage of dry matter, and the highest percentage of ash and of nitrogen in that dry matter. In the straw, too, the dry matter is low, the ash somewhat high, and. the nitrogen much the highest in the series. In 1845, another year of spring-sowing, and at the same time of very bad quality of produce, we have nevertheless a large amount of growth ; a fact vrhich tends to explain some of the differences in compositioii £|.s. gcijnpared with 1853. Thus, 1845 8 LAWES AND GILBERT gives US low percentage of dry matter, but riot very high, either ash or nitrogen, in the grain. The straw, however, gives high per^ centages both of ash and of nitrogen; it being in the latter point next in order to 1853. The seasons of 1848 and 1852 again show low characters of produce. The former has coincidently the lowest percentage of dry matter in the grain in the series ; and both have high percentage of ash and nitrogen in the dry sub- stance of the grain. In the straw, the ash is in 1848 the highest, and in 1853 above the average; the nitrogen in dry matter of straw being however in neither instance high. In several of the cases here cited, there are deviations from our general assumption on one point or other. But an examination, in greater detail, would in most or all of them clear up the appa- rent discrepancy. When indeed, we bear in mind how infinitely varied was the mutual adaptation of climatic circumstances to stage of growth of the plant, in almost every case, it would indeed be anomalous, did we not find a corresponding variation on some point or other, in the characters or composition of the crop. Still, we have the fact broadly marked, that within the range of our own locality and climate, high maturation of the wheat crop is, other things being equal, generally associated with a high percentage of dry substance, and a low percentage of both mineral and nitro- genous constituents. Were we, however, extending the period of our review, and going into detail as to varying climatic circum-. stances, interesting exceptions could be pointed out. It may be observed in passing, that owing to the general rela- tionships of the amounts of corn to straw, and the generally coin- cident variations in the percentages of nitrogen in each, the tendency of all these variations is in a degree so to neutralize each other, as to give a comparatively limited range of difi'erence in the figures, representing for each year, the percentage of nitrogen in the dry substance of the total produce — corn and straw together. The tendency of maturation, to reduce the percentages of mineral matter, and frequently of nitrogen also, is not observable in corn crops alone. We have fully illustrated it in the case of the turnip ; and our unpublished evidence in regard to some other crops, goes in the same direction. The fact is indeed very important to bear in mind ; for it constitutes an important item in our study of the variations which are found to exist in the composition both of the organic substance, and of the ash, of one and the same crop, grown under different circumstances. We may particularly observe, ON THE COMPOSITION OF WIIEAT-GUAIN, &Ci S that the obvious reduction in the percentage of nitrogen in wheat- grain, the more, within certain climatic limits, the seed is perfected, is in itself a fact of the highest interest j and it is the more so, when we consider how exceedingly dependent for full growth, is this crop upon a liberal supply of available nitrogen within the soil. Bearing in mind, then, the general points of relationship which have been established between the characters of the crop as to development and maturation on the one hand, and the percentage amounts of certain constituents on the other, let us now see — ^what is the general influence of characteristic constituents of manure, upon the characters and composition of our wheat crop, which is allowed to remain on the land until the plant has fulfilled its highest function — namely, that of producing a ripened seed ? In illustration of this point we have arranged in Table III, the same particulars as to general character of the crop, and as to the composition of the produce, from several individual plots during the ten years; instead of the average of the series in each year, as in Table I. The cases selected for the comparison are : — 1. A continuously unmanured plot ; 2. A plot having an excess of ammoniacal salts alone every year; 3. The average of several plots, each having the same amount of ammoniacal salts as the plot just mentioned, but with it, a more or less perfect provision by manure, of the mineral con- stituents also. It would be impossible to give the detail supplying all the results collected in this Table III ; but perhaps it is only proper that we should do so, so far at least as the percentage of nitro- gen in the dry substance of the grain is concerned. 10 LAWE8 AND GILBERT TABLE II. Determinations of Nitrogen per Cent, in the Dry Matter of Wheat Grain grown at Rothamsted. EXPEKIMBNTS. Harvests 1 2 3 i 5 Meau, TJnmaniired. 1845 2-28 2 '21 2-33 2-30 2-28 1846 2-11 2-12 .. , , 2-11 1847 2 11 2-08 2-22 2-22 2-16 1848 2-33 2-34 2-32 2-37 2-34 1849 1-85 1-83 1-91 .. 1-86 1850 2 07 210 2 07 2-08 .1851 1-80 1-74 1-89 1-76 1'80 1«52 2-31 2-23 2-33 2-31 2-31 1853 2-26 2-33 2-38 2-32 1854 2-06 2-06 1-98 1-96 2 01 Manured with Ammoniacal Salts only. 1845 2 18 2-29 2-22 2-23 2-23 1846 2 18 2-12 2-29 2-19 2 19 1847 2 36 2-29 2-42 2-32 2-34 1848 2 39 2-41 2 39 2-49 2-42 1849 1 89 2 04 1-92 1-95 1860 2 13 2-08 2-19 213 1851 2 15 2 12 2-09 2-25 2 15 1862 2 41 2-50 2-44 2-58 2 48 1853 2 43 2-48 2-37 2-44 2-43 1854 2-31 2-22 2-31 2 37 2-30 Manured with Ammoniacal Salts and Mineral Manure. (Mixed Plots.) 1845 1846 2-20 2-14 2 14 2 16 1847 2-34 2-38 2-40 2-42 2-44 2-40 1848 2-36 2-40 2-42 2-48 2-41 1849 1-96 1-97 2-10 2-07 2-02 1860 2-16 2-28 2-25 2-25 2 23 1861 2 00 1-98 2-02 1-92 1-98 1852 2-43 2-34 2-31 2-40 2-32 2-36 1853 2-30 2-34 2-29 2-28 2-30 1854 2-16 •• 2-12 2-07 •• 2-12 ON THE COMPOSITION OF WHEAT-GEAIN, &C. 11 It is necessary to make a few remarks in reference to this Table of more than one hundred nitrogen determinations. They were made by the method of burning with soda-lime, and collecting and weighing as platinum salt in the ordinary way. Few, perhaps, who have only made a limited number of such determinations, then only on pure and uniform substances, and who have not attempted to control their work at another period, with fresh re-agents, or by the work of another operator, will imagine the range of variation which is to be expected when all these adverse elements are to have their influence. It is freely granted, that the variations shown in the Table between one determination and another, on one and the same substance, are sometimes more than could be desired. The following, however, are the circumstances under which they have been obtained. Experiments 1 and 3 were pretty unifortaly made by the same operator, but not all consecutively, or with the same batch of re-agents. It was thought, therefore, that inde- pendently of .any variations between the two determination^, it would be desirable to have results so important in their bearings, verified by others. Accordingly, samples of each of the ground grains were given under arbitrary numbers, to two other operators, and their results are recorded respectively in columns 3 and 4 ; and where a fifth determination is given, it is a repetition by one or other of the experimenters last referred to. We should observe, that we have found it almost impossible to procure a soda-Hme that will not give more or less indication of nitrogen when burnt with an organic substance not containing it ; and hence we have at length adopted the plan of mixing 1-2 per cent, of non-nitro- genous substance intimately with the bulk of soda-lime, igniting it in a muffle, moistening, and reheating it gently. After this treatment the soda-lime is free from ammonia yielding matter. It should further be remembered, that a ground wheat-grain is by no means an uniform substance. Indeed, as we shall show further on, some of the particles of which such a powder is com- posed, may contain half as much again of nitrogen as-others ; and thus any inefficiency in the grinding, or error in taking the por- tion for analysis, may materially affect the result. Notwithstand- ing all these circumstances, and the admittedly undesirable range of difference in the several determinations in some cases, it wiU be observed, that generally three at least of the numbers agree sufficiently closely, and in some cases the fourth also. In fact after all, a study of the detailed table, must give considerable confidence, at least in the direction of the variations between the mean results given in Table III, and in their sufficiency for the arguments founded upon them. With these remarks on the data, let us proceed with the discussion of Table III itself, which next follows ; 12 LAWES AKD GILBERT M ffl •s lis- -omiuy ij 6[iij"ainp5 s e s o o o s s s is o o ? 8 o ^ O ■Xl«o o C^ ^ Ct
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ON THE COJfPOStTldi^ ^P WHEAt-GBAIN, &C. 13
A glance at this Table III, shows that the quantity of produce
varies very much indeed in one and the same season, according to
the manuring. With these great differences in the quantities,
dependent on manuring, we have far less marked differences in the
quality of this ripened crop, dependent on the same causes ; and
this, with some few exceptions, is the same whether we look to the
columns indicating the general characters only, or the composition
of the produce. That is to say, the same general distinctions
between the produce of one season and another, are observable
under the several varying conditions of manuring in each, as have
been exhibited in the Table I of averages alone. In fact, season,
or climatic variations, are seen to have much more influence than
manuring, upon the character and composition of the crop.
We have said that, other things being equal, the percentage
of nitrogen in our wheat-grain was the lower the more the seed
was perfected ; and we have also said, that nitrogenous manures
greatly aid the development of the crop. But, an inspection of
the columns of Table III which give the percentages of nitrogen
in the dry substance of the grains produced under the three
different conditions of manuring specified, shows us that there is
almost invariably, a higher percentaige of nitrogen where ammo-
niacal salts alone have been employed, than where the crop was
unmanured. We also see that, almost invariably, there is a higher
percentage of nitrogen where mineral manures as well as ammo-
niacal salts have been used, than in the produce of the corre-
sponding unmanured plots, A closer examination shows, however,
though the indication is not uniform, that there is nevertheless,
an obvious tendency to a lower percentage of nitrogen, where the
mineral constituents also have been employed, than where the
ammoniacal salts have been used alone ; and with this, there is on
the average, a somewhat higher weight per bushel, indicating
higher degree of maturation. Then, again, what are the circum-
stances of these experiments, under which an increased percentage
of nitrogen in the fixed substance of the produce, is obtained by
a supply of it in manure ? The unmanured plot with its low per-
centage of nitrogen in produce, is shown by the field experiments,
to be greatly exhausted of the annually available nitrogen, relatively
to the annually available mineral constituents required by the
wheat crop. The plot, with the ammoniacal salts alone, is shown
by the field results to be defective in the requisite and available
minerals, relatively to the available nitrogen, and hence the crop
14 LAWES ANP ^ILBEET
is grown under a rela,tive excess of the latter. Agaiii, the plots
•with mineral manures and ammoniaeal salts together^ received so
far an excess of the latter, as to yield, with the minerals, a larger
crop than the average of the locality under rotation, and larger
also, than the average of seasons would ripen healthily. It is then,
under these artificial and abnormal circumstances, of the somewhat
unnaturally low percentage of nitrogen, from obvious defect of it in
relation to the developing and maturing capabilities of the season
on the one hand, and the obviously relative excess of it on the
other, that we got an increased percentage of nitrogen in wheat-
grain by the use of it in manure. Even under these extreme
conditions, the range of variation by manuring is very small ; and
there is nothing in the evidence that justifies the opinion, that,
within the range of full crops and healthy maturation, the per-
centage of nitrogen in wheat grain, can be increased at pleasure by
the use of it in manure. That very opposite extremes of condition
of soil-supply, may directly influence the composition even of
wheat-grain, is however, illustrated in the percentages of mineral
matter, as well as those of nitrogen, given in the table. Thus,
taking the mean results only, we have with the relative excess of
mineral constituents on the unmanured plot, the highest per cent,
in the produce; with the greatest relative defect on the plot with
ammoniaeal salts only, the lowest per cent, in the grain ; and with
. the medium relation in the other plots, the medium per cent, in
the produce. Excepting, however, abnormal conditions, as already
remarked, variation in climatic circumstances, has much greater
influence on the percentage-composition of wheat-grain, than
variation in manuring.
Let us now turn to the composition of the ash of wheat-grain.
Independently of the defect of a sufiicient number of published
analyses of wheat-grain ash, a dozen years ago, when we took up
the subject, it was then generally believed that the composition
of the ash of vegetable produce, would vary considerably with
the supplies of the different constituents in the soilj it was
thought indeed, that according to the abundance of their presence,
one base might substitute another, as for instance soda, potash,
and so on. About the same time that we undertook a series of
wheat-ash analyses, the ashes of various succulent vegetables were
also analysed. This latter investigation led us to conclude, that the
fixity of the composition of the ash of such substances, depended
very much upon the degree of niatura,tion of the produce ; and in
ON THE COMPOSITJON OP WHEAT-GKAIN, &C. 15
fact that ' sojne constituent^'^soda ^od chlorine for ^nstancgTr.,-
occurred in much larger quantities in the more succulent aijd
unripe, than in the more elaborated specimens. It seemed to he
perfectly consistent with thig experience, to find in the jish of a
comparatively perfected vegetable product like wheatrgrain, a con-
siderable uniformity of composition — such indeed as the analyses
no^ to be recorded will indicate.
These analyses were made ten years ago by Mr. Dugald
Campbell, and the late Mr. Ashford. And as, since that time,
the methods of ash-analysis have in some points been improved
upon, it will be weU to give an outline of the plan then adopted :
especially as it is by a consideration of the tendencies to error on
some points, that we must interpret the bearings of the actual
figures given. On this point we need only add, that Mr. C a pip-
bell fully concurs in the tenor of our remarks.
Method of Analysis : — Three portions of ash were taken.
No. 1. In this the sand, silica, and charcoal, phosphate of iron,
phosphoric acid, lime, and magnesia, were determined, The ash
was dissolved in dilute hydroghloric acid, evaporated to perfect
dryness, moistened with hydrochloric acid, boiled with water, and
the insoluble matter collected and weighed, as — sand, silica, and
charcoal. To the filtrate, acetate of ammonia was added, and
after digestion, the precipitate separated, dried, ignited and weighed
— as phosphate of iron. To the filtrate now obtained,' a solution
of a weighed portion of pure iron dissolved in nitro-hydrochloric
acid was added, then acetate of ammonia, and the mixture
digested until the whole of the iron was precipitated as phosphate
of the peroxide with excess of peroxide, from which was calculated
the phosphoric acid. From the solution filtered from the phos-
phate of iron and oxide of iron, the lime was separated as oxalate
and ignited as carbonate; and from this last filtrate, the magnesia,
by phosphate of soda and ammonia.
No. 2. A second portion of ash was put into a carbonic acid
apparatus, the acid, if any, evolved by means of nitf ic acid, and
determined by the loss. The solution being filtered, sulphuric
acid was separated by nitrate of baryta ; and afterwards chlorine
by nitrate of silver.
No. 3. To a solution of a weighed portion of the ash in
hydrochloric acid, caustic baryta was added in excess, and the
precipitate separated by filtration ; the excess of baryta was then
16 lAWES AND GILBERT
removed fey carbonate of ammonia, and the filtered solution
evaporated to dryness, the residue heated to redness and weighed ;
"water added, any insoluble matter deducted, and the remainder
taken as chlorides of potassium and sodium ; a solution of chloride
of platinum was now added to separate the potash; the soda being
calculated from the loss.
It is now admitted, that the separation of phosphate of iron
from the earthy phosphates by acetate of ammonia as above
described, is unsatisfactory ; and it is probable the amounts given
in the tables as phosphate of iron are too high, and if so, part of
the difference should obviously go to the earthy bases. For a
similar reason it is possible that the phosphoric acid determinations
may be somewhat too high — also at the expense of the earthy
bases. Then again, it is well-known that in practice the process
for potash and soda, is one of some delicacy ; and that the tendency
of manipulative error is to give the soda somewhat too high. We
conclude upon the whole, that our phosphoric acid determinations
may be somewhat high ; our phosphate of iron pretty certainly
so ; and probably the soda also ; the other bases being, on this
supposition, given somewhat too low.
The wheat-grain ash-analyses, 23 in number, and referring to
the produce of three separate seasons, and of very various manur-
ing, are given in the following Tables — numbered IV, V and VI
respectively.
ON THE COMPOSITION OP WHEAT-GEAIN, &C.
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